ArticleAngewandte Chemie (International ed. in English)2026
Surface Chemical Disorder Engineering Enabled Superior Anion Redox for Li-Rich Mn-Based Cathode.
Article in Angewandte Chemie (International ed. in English), 2026. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Not yet cited in PubMed.
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Abstract
The Li-rich Mn-based oxides have attracted extensive attention due to the specific anion redox reaction to provide high capacity. However, the poor reversibility of anion redox leads to serious lattice oxygen loss and surface structure evolution. Here, we report an approach by integrating chemical disorder-based crystallographic texture into the cathode surface to solve these questions, which involves the spatial rearrangement of lattice oxygen by supersaturated occupation of cations in the lattice. This makes the oxygen electronic structure delocalized and diversified, strengthens the metal-oxygen orbital hybridization, and effectively improves the reversibility and kinetics of anion redox reactions. Meanwhile, the robust surface architecture effectively inhibits superficial detrimental phase evolution and electrode/electrolyte interface side reactions, maintaining the structural integrity of the electrochemical process. Accordingly, the as-designed modified cathode delivered a promising capacity (291.8 mAh g
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