ArticleAngewandte Chemie (International ed. in English)2026
Design Guidelines for Anode Modifications to Eliminate Soft Short Circuits in Anode-Free Na Batteries Under High Current Density With Large-Capacity Plating, Demonstrated via Initiated Chemical Vapor Deposition (iCVD).
Article in Angewandte Chemie (International ed. in English), 2026. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Not yet cited in PubMed.
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Abstract
Soft short circuits, an underrecognized failure mode, are especially critical in anode-free sodium systems, where limited Na inventory makes cells highly vulnerable to irreversible Na loss. However, clear interphase-design principles for suppressing soft shorting remain lacking because its interfacial origin and governing descriptors are still poorly understood. Herein, we propose a mechanistically guided interphase design strategy for soft-short-free Na metal anodes under practical conditions. An ultrathin (20 nm) poly(1H,1H,7H-dodecafluoroheptyl acrylate) (pDFHA) layer was conformally deposited on an Al current collector via a solvent-free vapor-phase polymerization process. Its minimal thickness and intrinsic ionic conductivity enabled favorable Na
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