ArticleChemistry (Weinheim an der Bergstrasse, Germany)2026
pH-Dependent Photosensitized Generation of Multiphase •OH Radicals: Unravelling the Catalytic Mechanism.
Article in Chemistry (Weinheim an der Bergstrasse, Germany), 2026. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Not yet cited in PubMed.
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Abstract
Photosensitized reactions at aerosol interfaces are pivotal to regional atmospheric oxidizing capacity, but the complex physicochemical architecture of atmospheric particles severely impedes mechanistic elucidation of photochemical pollution. We report that polycyclic aromatic hydrocarbons (PAHs) in soot photosensitization processes can function as critical catalysts driving hydroxyl radicals (•OH) formation. Photochemical experiments and quantum-chemical calculations reveal that photoexcited PAHs activate two distinct •OH generation channels. On the one hand, the conversion of excited-state PAHs to •PAH
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