ArticleNature communications2026
Adsorption based on excitation.
Article in Nature communications, 2026. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Not yet cited in PubMed.
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Authors and funding
7 authors.
Funding
Abstract
Traditionally, adsorption is believed to take place only in the ground state, but here we report an excitation-driven adsorption mode. Composites of metallophthalocyanines and carbonaceous substrates are prepared, among which the potassium-phthalocyanine (KPc)/reduced graphene oxide (RG) composite shows the most typical behavior. Femtosecond transient absorption spectroscopy and first-principles simulations reveal that under ultraviolet (UV) irradiation, the excited electrons in the composite transfer efficiently from KPc to RG, leaving long-lived excited holes on KPc that enable selective adsorption of CO molecules. In the dark, the composite shows negligible CO adsorption (0.06 mmol g⁻
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