ArticleACS central science2026
Theoretically Unveiling the Factors That Control Activated Ion Mobility in Lithium-Based Polymerized Ionic Liquids and Glasses.
Article in ACS central science, 2026. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Not yet cited in PubMed.
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5 authors.
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Abstract
Understanding the activated transport of ions in neat polymeric liquids and glasses is a fundamental scientific problem in materials, polymer, and physical chemistry, and it is highly relevant for diverse energy storage applications. Of special interest are cation-based single ion conductors, "polymerized ionic liquids" (PolyILs). We combine three recent advances in microscopic statistical mechanical theory for multiscale structure, ion hopping, and polymer segmental dynamics to address how structural correlations, thermodynamic state, and anion-cation association strength determine the temperature-dependent activation barrier for ion transport and its coupling with polymer motion. The key is a new mapping of molecular complexity to a coarse grained model that encodes the chemically specific glass transition temperature,
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