ArticleAdvanced materials (Deerfield Beach, Fla.)2026
Orbital-Hybridizable Nanoseed Interphase Enables One-Minute Rechargeable, Energy-Dense Anode-Free Aqueous Zinc Batteries.
Article in Advanced materials (Deerfield Beach, Fla.), 2026. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Not yet cited in PubMed.
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Abstract
Aqueous zinc (Zn) batteries are emerging as promising candidates for energy storage systems (ESS) and wearable electronics, but their practical application is hindered by low energy density and electrochemical instability at the Zn anode-electrolyte interface. Here, we report an orbital-hybridizable nanoseed (OHNS) interphase composed of graphene oxide nanoribbons (GONRs) uniformly deposited on Cu current collectors via a scalable slot-die coating process, enabling one-minute-rechargeable, energy-dense anode-free aqueous Zn batteries. The carbon edges (C-edges) prevalent in the GONR facilitate orbital hybridization with Zn. This chemical interplay between the heteroatoms (C-edge and Zn) enhances Zn nucleation kinetics and retards surface diffusion of adsorbed Zn, thereby promoting corrosion-resistant, (002)-oriented growth of Zn. Consequently, reversible Zn plating/stripping with high Coulombic efficiency (∼99.5%) was achieved even at a high current density of 120 mA cm
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