ArticleAngewandte Chemie (International ed. in English)2026
Self-Limiting Covalent Ligation Mechanism Enabling Anomalously High Interfacial Compatibility in Organic-in-Sulfide All-Solid-State Lithium Batteries.
Yan Zhang, Yuxi Zhong, Ruiqi Guo, Songjie Li, Kaidi Kang, Bingguang Ye, Wei Shan, Ran Zhao, Xinran Wang, Chuan Wu and 1 more
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In one paragraphArticle in Angewandte Chemie (International ed. in English), 2026. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Not yet cited in PubMed.
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11 authors.
Yan ZhangBeijing Key Laboratory of Environmental Science and Engineering, School of Materials Science and Engineering, Beijing Institute of Technology, Beijing, People's Republic of China.
Yuxi ZhongBeijing Key Laboratory of Environmental Science and Engineering, School of Materials Science and Engineering, Beijing Institute of Technology, Beijing, People's Republic of China.
Ruiqi GuoBeijing Key Laboratory of Environmental Science and Engineering, School of Materials Science and Engineering, Beijing Institute of Technology, Beijing, People's Republic of China.ORCID https://orcid.org/0009-0006-3581-6327 Songjie LiBeijing Key Laboratory of Environmental Science and Engineering, School of Materials Science and Engineering, Beijing Institute of Technology, Beijing, People's Republic of China.
Kaidi KangBeijing Key Laboratory of Environmental Science and Engineering, School of Materials Science and Engineering, Beijing Institute of Technology, Beijing, People's Republic of China.
Bingguang YeBeijing Key Laboratory of Environmental Science and Engineering, School of Materials Science and Engineering, Beijing Institute of Technology, Beijing, People's Republic of China.
Wei ShanBeijing Key Laboratory of Environmental Science and Engineering, School of Materials Science and Engineering, Beijing Institute of Technology, Beijing, People's Republic of China.
Ran ZhaoBeijing Key Laboratory of Environmental Science and Engineering, School of Materials Science and Engineering, Beijing Institute of Technology, Beijing, People's Republic of China.
Xinran WangBeijing Key Laboratory of Environmental Science and Engineering, School of Materials Science and Engineering, Beijing Institute of Technology, Beijing, People's Republic of China.ORCID https://orcid.org/0000-0002-2911-9051 Chuan WuBeijing Key Laboratory of Environmental Science and Engineering, School of Materials Science and Engineering, Beijing Institute of Technology, Beijing, People's Republic of China.ORCID https://orcid.org/0000-0003-3878-179X Ying BaiBeijing Key Laboratory of Environmental Science and Engineering, School of Materials Science and Engineering, Beijing Institute of Technology, Beijing, People's Republic of China.ORCID https://orcid.org/0000-0003-3645-4357 Funding
Beijing Natural Science Foundation L247017Fundamental Research Funds for the Central Universities 2024CX06061National Natural Science Foundation of China 22379016National Program of China, the National Key Research and Development Program of China 2022YFB2404400
6 · The paper itselfAbstract
Polymer-in-sulfide composite electrolytes have emerged as highly promising candidates for all-solid-state lithium batteries (ASSLBs) due to their on-demand shaping and rapid ion diffusivity. However, a striking paradox arises in the case of ethylene oxide-tethered polyacrylates (EO-PAs): their high polarity/strong nucleophilic tendencies constitute a major threat to sulfide stability yet exhibit anomalously high polymer/sulfide compatibility in practice. The underlying mechanism remains a matter of uncertainty. Herein, we first reveal a self-limiting covalent ligation mechanism that accounts for this compatibility paradox. Central to this principle is the identification of intimate interactions between terminal -CH
Indexed as
interface stabilitypolymersself‐limiting covalent ligationsolid electrolytessulfides
Identifiers
PMID42189699
PMCPMC13383021
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