ArticleNpj biosensing2026
Metal-phenolic networks improve interfacial electron transfer in bio-electrochemical systems.
Article in Npj biosensing, 2026. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Not yet cited in PubMed.
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6 authors.
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Abstract
Multi-enzyme electrocatalytic cascades often suffer from poor electron-transfer efficiency, limiting their utility. We overcome this critical challenge by integrating an interfacial metal-phenolic network (MPN) layer with tunable properties based on the metal and polyphenol employed. Upon electropolymerization, MPNs provide a stable matrix for co-immobilizing glucose oxidase and horseradish peroxidase, enhancing their tandem activity. Through systematic evaluation of the impact of MPN composition on electron transfer, we demonstrate the tunability of these materials for cascade-specific optimization. This simple material is expected to support diverse enzymatic reactions important for technologies ranging from bioenergy to biosensing.
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