ArticleSmall (Weinheim an der Bergstrasse, Germany)2026
Robust Liquid-Free Supramolecular Ionic Conductive Elastomers Enabled by Hierarchical Hydrogen-Bond-Induced Soft Crystalline Strategy for Fiber Electronics.
Article in Small (Weinheim an der Bergstrasse, Germany), 2026. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Not yet cited in PubMed.
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Abstract
Fiber electronics that can be miniaturized and seamlessly integrated onto the soft and dynamically deforming human body are emerging as a transformative class of wearable technologies. However, as an indispensable key material, ion conductors face an inherent trade-off between covalent rigidity and dynamic energy dissipation, making it difficult to achieve spinnability and durability. Herein, a soft crystalline strategy based on dynamic hydrogen-bond-induced microcrystalline fracture within polymers is developed to integrate mechanical robustness into stretchable ionic conductors. The molecularly programmed elastomeric matrix contains hierarchical hydrogen bonds spanning a wide energy range, which enable dynamic stretchability through reversible dissociation and reformation, while these hydrogen bonds and the induced microcrystalline fragments synergistically enhance the robustness of ionic conductors. The obtained ionic conductive elastomer exhibits an exceptional combination of stretchability (804.8%), tensile strength (2.2 MPa), and toughness (15.8 MJ m
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