ArticleNature communications2026
Strongly-coordinating organoborates with eccentric solvation structure enable secondary calcium metal battery.
Article in Nature communications, 2026. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Not yet cited in PubMed.
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Abstract
Rechargeable calcium (Ca) metal batteries are promising candidates for next-generation energy storage owing to calcium's abundance, divalent charge and low redox potential. However, achieving reversible Ca plating/stripping at room temperature remains challenging due to sluggish desolvation kinetics and unstable interfacial chemistry. Here, we design a class of reversible calcium electrolytes using eccentric solvation structure strategy by introducing strongly coordinating monovalent organoborates into calcium-based electrolytes. The tetra(trifluoroethanoloxy)-borate anion enables participation in the primary solvation sheath, while monovalent cations promote the formation of eccentric solvation structures via anion bridging. This solvation environment lowers both the solvation sheath reorganization energy and desolvation energy barrier of Ca
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