ReviewChemistry (Weinheim an der Bergstrasse, Germany)2026
Topology-Engineered Three-Dimensional Porphyrin-Based Covalent Organic Frameworks for Photo- and Electrocatalysis.
Review in Chemistry (Weinheim an der Bergstrasse, Germany), 2026. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Not yet cited in PubMed.
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The abstract states no effect estimate the extractor could read, or names no intervention and outcome on the map, so this paper lights no cell and moves no belief. It is still indexed, cited and linked below.
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4 authors.
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Abstract
Photo- and electrocatalytic conversion of abundant resources into value-added chemicals is a promising route to address rising energy demands and environmental sustainability. Achieving high efficiency requires catalysts that promote rapid charge generation, separation, and transport. Porphyrin-based covalent organic frameworks (Por-COFs) provide well-defined modular architectures with tunable electronic structures. Although two-dimensional (2D) Por-COFs can offer fast in-plane charge transport via extended π-conjugation, their densely stacked layers often impede mass diffusion and limit interlayer charge migration. By contrast, three-dimensional (3D) Por-COFs feature interconnected open channels and fully exposed active sites, enabling efficient charge separation, multidirectional charge transport, and improved accessibility of reactants and guests. These attributes translate into enhanced photo- and electrocatalytic activity. This article summarizes recent progress in the design and catalytic applications of 3D Por-COFs, emphasizing topology-guided structural engineering, performance optimization strategies, and structure-property-activity relationships. Remaining challenges and future opportunities are discussed to guide mechanistic understanding and accelerate practical implementation.
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