ReviewNature protocols2026
SMAIS: a universal platform for the on-water surface synthesis of two-dimensional polymer crystals.
Review in Nature protocols, 2026. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Not yet cited in PubMed.
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Abstract
Two-dimensional polymers (2DPs) are covalent polymeric networks with intrinsic long-range order in two orthogonal directions. Their unique physicochemical properties include tunable opto-electronic properties, mechanical stability and precisely defined nanopores that enable ion and molecular sieving. Here we describe a universal approach for the precise synthesis of 2DPs through the surfactant-monolayer-assisted interfacial synthesis method. The surfactant-monolayer-assisted interfacial synthesis combines the on-water surface reactivity and the role of surfactant (for example, sodium oleyl sulfate and sodium dodecyl benzenesulfonate) to guide the monomer-programmed assembly, two-dimensional (2D) polymerization and crystallization processes on the water surface, yielding large-area and highly crystalline 2DPs. This versatile Protocol has been used to synthesize many 2DP crystals, including 2D polyamide, 2D polyimide, 2D polyimine, 2D poly(boronate ester), 2D poly(pyridinium salt), 2D polyphenylenevinylene, 2D polybenzimidazole and 2D polyaniline, with a large lateral size of ~28 cm
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