ArticlePloS one2026
Thiol-functionalized ZrP reinforced poly(MMA-co-MI) nanocomposites: High optical transparency and superior thermal stability for optical coatings.
Article in PloS one, 2026. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Not yet cited in PubMed.
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Abstract
This study presents novel transparent and thermally stable nanocomposites based on poly(methyl methacrylate-co-N-2-methyl-4-nitrophenylmaleimide) (P(MMA-co-MI)) reinforced with thiol-functionalized zirconium phosphate (ZrP-SH) nanofillers. The key innovation is the thiol modification of ZrP, which enhances interfacial interactions and ensures uniform dispersion at low loadings (≤1 wt%). The nanocomposites were prepared through solution blending and characterized using FTIR, XRD, SEM, TEM, TGA, DSC, and UV-Vis spectroscopy. Compared to the neat copolymer, the nanocomposites demonstrated an approximately 30 °C increase in glass transition temperature (from 164.3 °C to 168.4 °C) and an increase in onset degradation temperature from 265 °C to about 297 °C while maintaining high optical transparency in the visible range at low filler contents. These silicon-free materials effectively address the trade-off between thermal stability and optical clarity, offering significant potential for advanced optical coatings, sensors, protective layers, and optoelectronic packaging applications.
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