ArticleSmall (Weinheim an der Bergstrasse, Germany)2026
Supramolecular Chiral Assembly of Open-Shell Quinoids With Chiral Additives and Their Spin-Dependent Transport in Magneto Field-Effect Transistors.
Article in Small (Weinheim an der Bergstrasse, Germany), 2026. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Not yet cited in PubMed.
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Abstract
Chiral conjugated materials stand at the forefront of organic electronics because of their chiroptical properties and spin-filtering capabilities. Although chiral materials with intrinsic spins show significant promise for organic spintronics, their development remains challenging due to structural and assembly constraints. In this study, a series of quinoid molecules with intrinsic spins (QFn) is developed and assembled into chiral supramolecular structures by blending with the chiral additive 1,1'-binaphthyl-2,2'-diamine (BN). Chirality transfer is considered to occur through F···H-N hydrogen bonding, and succeeds only in fluorinated QF1 and QF2. Thermal annealing yields markedly different degrees of chirality amplification, depending on the molecular structure. Asymmetric QF1 forms stable co-crystals with BN, resulting in a 30-fold amplification of chirality with an absorption dissymmetry factor (g
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