ArticleChemistry (Weinheim an der Bergstrasse, Germany)2026
Polarity on Demand: Nucleophilic, Electrophilic, and Ambiphilic Reactivity at a 9,10-Dihydro-9,10-Disilaanthracene Platform.
Article in Chemistry (Weinheim an der Bergstrasse, Germany), 2026. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Not yet cited in PubMed.
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5 authors.
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Abstract
9,10-Dihydro-9,10-diheteroanthracenes constitute rigid molecular entities that enable cooperative reactivity between two proximal heteroatoms. While diboraanthracenes act as ditopic Lewis acids and diphosphaanthracenes as ditopic Lewis bases, ambiphilic behavior has so far largely relied on the incorporation of two different heteroelements. Herein, we demonstrate ambiphilicity within a homo-heteroelement framework based on 9,10-dihydro-9,10-disilaanthracene (DSA). Efficient cyclocondensation of 1,2-disilyl-4,5-dimethylbenzene, promoted by substoichiometric amounts of MeLi, affords DSA 1
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