ArticleAdvanced science (Weinheim, Baden-Wurttemberg, Germany)2026
A New Customizable Surfactant LLPS Strategy for Sustainable and Highly Efficient Radioactive Metal Ion Separation.
Article in Advanced science (Weinheim, Baden-Wurttemberg, Germany), 2026. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Not yet cited in PubMed.
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Abstract
The traditional aqueous-organic biphasic extraction for separating radioactive metal ions faces major challenges due to heavy reliance on volatile organic solvents and the resulting refractory radioactive waste. Herein, we propose a customizable, sustainable, and efficient separation strategy for radioactive ions by using liquid-liquid phase separation (LLPS) phenomenon in two coexisting aqueous phases. Unlike conventional organic extraction systems, the LLPS platform operates without forming a bulk organic extraction phase. The LLPS is formed by sodium dodecyl sulfate (SDS), cetyltrimethyl ammonium bromide (CTAB), and hexafluoroisopropyl alcohol (HFIP) (termed as SCH-extraction system) and enables customized encapsulation of commercial extractants. The selectivity of SCH-extraction system can be precisely tuned by adjusting parameters like the type of extractant and solution acidity, making it highly versatile for various separation scenarios. In simulated high-level liquid waste (HLLW), the strategy achieved the separation factors of
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