ArticleMaterials horizons2026
Synthesis and pyroelectric response of disperse red 1 functionalized silicones: cyclic monomer, homopolymer, and block copolymer derivatives.
Article in Materials horizons, 2026. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Not yet cited in PubMed.
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Abstract
Pyroelectric materials enable the direct conversion of thermal fluctuations into electrical energy, offering a promising approach to waste heat recovery. While pyroelectric polymers are highly valued for their scalable synthesis, mechanical flexibility, and tunable properties, the field is currently dominated by poly(vinylidene fluoride) (PVDF)-based materials, which present environmental and processing challenges. To develop fluorine-free alternatives and elucidate the influence of molecular architecture on thermal-to-electrical conversion, we synthesized a series of siloxane-based materials functionalized with Disperse Red 1 (DR1) moieties, including a cyclic siloxane monomer, a homopolysiloxane, and a block copolysiloxane. Differential scanning calorimetry confirms the semicrystalline nature of these siloxanes, with glass transitions (
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