ArticleJournal of the American Chemical Society2026
Kosmotrope-Promoted Proton Hopping in Supramolecular Conductors.
Article in Journal of the American Chemical Society, 2026. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Not yet cited in PubMed.
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7 authors.
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Abstract
Scientific interest in the Hofmeister effect has waxed and waned since its discovery over a century ago; however, its ion-specific influence on solvation and molecular organization remains a topic of enduring significance. While extensively studied in aqueous systems, its relevance to solid-state materials and Grotthuss mechanisms has remained largely unexplored. Here, we unveil a class of supramolecular organic cage salts, the Cage1 series, with counteranions spanning the Hofmeister series to systematically probe their ion-specific effects on solid-state proton conduction. Kosmotropic anions, stabilized by the supramolecular organic cage, are found to markedly enhance proton conductivity, promoting the formation of an extended hydrogen-bonded network (HB-network) that facilitates Grotthuss-type proton hopping. The conductivity increases by over 2 orders of magnitude from chaotropic Cage1-HI to kosmotropic Cage1-H
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