ArticleJournal of the American Chemical Society2026
Chemical Engineering of Altermagnetism in Two-Dimensional Metal-Organic Frameworks.
Article in Journal of the American Chemical Society, 2026. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 1 paper.
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Who cites it
1 citing paper in PubMed.
- Altermagnetic Metal-Organic Frameworks.Journal of the American Chemical Society · 2026Review
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Authors and funding
4 authors.
Funding
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Abstract
Altermagnetism represents a novel magnetic phase exhibiting nonrelativistic spin splitting without net magnetization driven by lattice symmetry. Here, we introduce a general coordination-chemistry-based strategy to realize and control altermagnetic (AM) spin splitting in two-dimensional (2D) planar tetracoordinated Cr-based metal-organic frameworks (MOFs). Using density functional theory (DFT) calculations, we demonstrate that ligand symmetry and its arrangement within the lattice can be used to lower the crystallographic symmetry of Cr-based MOFs, enabling g-wave AM spin splitting up to 65 meV. Furthermore, frontier molecular orbital engineering (FMOE) allows selective ligand spin polarization, inducing a shift to d-wave AM anisotropy in polycyclic ligand-based 2D MOFs with spin splitting up to 83.9 meV. Microscopic magnetic exchange interaction (
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Registered trials
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