Evidence map›Paper›PMID 42130155›Full record

ArticleJournal of environmental quality

Designing biochars for improved sorptive removal of per- and polyfluoroalkyl substances.

Wei Zheng, Erin Huggett, Sophie Circenis, Kalidas Mainali, Brajendra Sharma

Abstract read
In one paragraph

Article in Journal of environmental quality. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 1 paper.

0numbers the graph read from it
0cells of the map it votes in
1citing papers in PubMed
–field-weighted citation impact
1 · What the graph read from it

What it found

Each row is one number read from the abstract, on the scale the paper reported it, with its interval. Left of the dashed line favours the treatment, right favours the comparator. Under each row is the sentence it came from. New to these charts? A ten-minute tutorial.

The abstract states no effect estimate the extractor could read, or names no intervention and outcome on the map, so this paper lights no cell and moves no belief. It is still indexed, cited and linked below.

2 · The registry

The trial behind it

Trials whose registry record cites this paper, or whose number appears in the abstract. A trial that started after this paper was published is citing it as background, not reporting it.

Neither the registry nor the abstract names a trial number. If this is a trial report, that itself is worth knowing.

3 · Its place in the literature

Who cites it

1 citing paper in PubMed.

  1. Article
4 · The record

Corrections and comments

PubMed lists nothing against this paper. Absence here is not a guarantee, only a check that was made.

5 · Who and what money

Authors and funding

5 authors.

Wei ZhengIllinois Sustainable Technology Center, University of Illinois at Urbana-Champaign, Champaign, Illinois, USA.ORCID https://orcid.org/0000-0002-0307-0915
Erin HuggettIllinois Sustainable Technology Center, University of Illinois at Urbana-Champaign, Champaign, Illinois, USA.
Sophie CircenisIllinois Sustainable Technology Center, University of Illinois at Urbana-Champaign, Champaign, Illinois, USA.
Kalidas MainaliUSDA-ARS Eastern Regional Research Center, Sustainable Biofuels and Co-Products Research Unit, Wyndmoor, Pennsylvania, USA.
Brajendra SharmaUSDA-ARS Eastern Regional Research Center, Sustainable Biofuels and Co-Products Research Unit, Wyndmoor, Pennsylvania, USA.

Funding

EPA R840952Strategic Environmental Research and Development Program (SERDP) ER22-3157
6 · The paper itself

Abstract

The widespread occurrence of per- and polyfluoroalkyl substances (PFAS) in aquatic environments, along with their adverse impacts on human health, has been recognized as an emerging issue. Sorption using carbon-based sorbents is the most common approach for PFAS removal. However, conventional biochars typically underperform compared to activated carbon, which is effective but relatively costly. In this study, a designer biochar was developed by using lime sludge, a no-cost byproduct from drinking water treatment plants, as a pretreatment for woody biomass followed by systematic optimization of lime-sludge loading, pyrolysis temperature, and residence time. The results showed that the pretreatment process enhanced pore development and modified the surface chemistry of the designer biochar. Under optimal conditions (1:4 lime sludge-to-biomass, 850°C, 5 h), the designer biochar achieved near-quantitative removal (>99%) of perfluorooctanoic acid and both linear and branched perfluorooctane sulfonate, outperforming unmodified biochar and comparable to a commercial activated carbon. Sorption kinetics and isothermal studies confirmed the superior performance of the designer biochar, exhibiting rapid equilibration (<1 h) and increased sorption capacity. Mechanistic analysis revealed that improved PFAS removal by the designer biochar was driven by multiple adsorption mechanisms, including hydrophobic interactions, electrostatic attraction, and cation bridging facilitated by Ca

Indexed as

Alkanesulfonic AcidsCaprylatesCharcoalFluorocarbonsWater Pollutants, ChemicalWater PurificationAdsorptionModels, ChemicalAlkanesulfonic AcidsbiocharCaprylatesCharcoalFluorocarbonsperfluorooctane sulfonic acidperfluorooctanoic acidWater Pollutants, Chemical

Identifiers

PMID42130155
PMCPMC13172648

What OpenQuestion holds

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LicenceCC BY
Read underepoch 390

Registered trials

None linked

Read under generation 80e0d062 · epoch 390. Bibliography from PubMed, PubMed Central and OpenAlex; grants from NIH RePORTER; trial links from ClinicalTrials.gov; estimates, votes and beliefs from the OpenQuestion graph.