ArticleChemSusChem2026
Polyampholyte Copolymers Based on Dual Ionic Monomers as Self-Healing Aqueous Binders for Lithium Ion Battery Cathodes.
Article in ChemSusChem, 2026. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Not yet cited in PubMed.
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7 authors.
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Abstract
Self-healing polymeric binders play a key role in preserving the mechanical stability of electrodes, as they can autonomously recover from mechanical damage, such as cracks or ruptures, without affecting battery performance. Herein, a polyampholyte copolymer family is designed with tunable glass transition temperature and self-healing properties associated with the reversible ionic and hydrogen bonding interactions. A dual ionic monomer (DIM) is synthesized by a proton transfer reaction between methacrylic acid (MA) and dimethylaminoethyl methacrylate (DMAEMA). A series of copolymers with both anionic and cationic groups in the polymer backbone were then synthesized by copolymerization of the DIM with poly(ethylene glycol) methyl ether methacrylate (PEGMEMA) at different ratios by free-radical polymerization in water. The poly(MA-co-DMAEMA-co-PEGMEMA) random copolymers presented different glass transition temperatures (T
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