ArticleAngewandte Chemie (International ed. in English)2026
Selective Nitrate Transmembrane Transport Through Adaptive Weak C─H Bonding Cyanostilbene Water Channels.
Article in Angewandte Chemie (International ed. in English), 2026. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Not yet cited in PubMed.
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Abstract
Transmembrane water transport strongly depends on how dynamic, translocating water clusters are stabilized within hydrogen-bonding (HB) channels. Both structural order and short-lived disorder of transient channels play important roles in ion and water translocation. Strong HB can result in tight water binding and reduced mobility. We hypothesize that weaker HB binding sites reduce water friction, thereby enhancing water permeation while suppressing ion transport due to their unmet dehydration requirements within membrane. Herein, we show that weak HB CH donor cyanostilbenes promote water transport through adaptive, less-ordered water channels within the lipid bilayer, with water translocation efficiency depending in part, on the strength of the CH donor sites. Fine-tuning both CH donor strength and binding geometry enables modulation of anion transport selectivity, ranging from moderate NO
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