ArticleAdvanced science (Weinheim, Baden-Wurttemberg, Germany)2026
Rational Design of Weakly-Solvating Molecules for Salt-In-Pre-Ionic-Liquid Electrolytes for Li Metal Batteries.
Article in Advanced science (Weinheim, Baden-Wurttemberg, Germany), 2026. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Not yet cited in PubMed.
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Abstract
Lithium metal batteries (LMBs) promise step-changes in energy densities but suffer from poor cycle life due to unstable electrolyte-lithium interfaces. Conventional carbonate electrolytes exhibit excessive lithium-ion solvation and low oxidative stability, leading to rapid capacity loss. Herein, we report a rationally designed weakly-solvating cyclic sulfonamide, 1-trifluoromethanesulfonyl)amide pyrrolidine (TFMSPyr), which integrates an electron-withdrawing trifluoromethanesulfonyl functional group at pyrrolidinic-N. TFMSPyr acts as a pre-ionic-liquid solvent that forms intrinsically localized, anion-dominated solvation, coupling molecular architecture, solvation topology, and transport dynamics. As a result, LiFSI based salt-in-pre-ionic-liquid (SIPIL) electrolytes exhibit high lithium-ion transference number, oxidative stability > 5 V versus Li/Li
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