ArticleChemical science2026
Rational design of pigment-polymer antenna complexes.
Article in Chemical science, 2026. The graph could read no effect estimate from its abstract, so it casts no vote on the map. An erratum has been issued. Not yet cited in PubMed.
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Corrections and comments
- Erratum issued
Authors and funding
12 authors.
Funding
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Abstract
We report the synthesis of biomimetic programmable pigment-polymer antenna complexes (PPACs) by using reductive amination to bind amine-functional dyes to surface-grafted aldehyde-functional PAGEO5MA chains grown from planar substrates by atom-transfer radical polymerization. The fraction of dye-conjugated repeat units can approach unity under optimized conditions. Dye binding kinetics are strongly influenced by steric factors and can be controlled by varying the polymer grafting density, the dye size and the nucleophilicity of its amine group. Absorption and fluorescence spectra of PPACs produced by conjugating Nile Red ethylamine (NRet) to PAGEO5MA brushes are sensitive to the dielectric environment within the layer. At low dye concentrations, the mean fluorescence lifetime
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Registered trials
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