Spin and Orbital Angular Momentum Polarization in Thouless Topological Charge Pumping.

Quantized charge pumping in one-dimensional chiral wires has been widely studied in the context of topological physics in (1 + 1)-dimensional synthetic space, yet the role of orbital and spin degrees of freedom remains largely unexplored. Here, we show that topological charge pumping in insulating chiral systems intrinsically generates orbital and spin polarization, providing a new perspective on spin-selective transport in chiral materials, often associated with chirality-induced spin selectivity. Using time-dependent Schrödinger dynamics of multiorbital tight-binding models driven by circularly polarized light, we identify two key results. First, the screw-like geometry enables a single-parameter topological charge pumping. Second, while the energy gap remains open throughout the pumping cycle, Berry phase driven dynamics induces nonequilibrium orbital polarization. Through spin-orbit coupling, this orbital response is partially converted into spin polarization. By analogy between synthetic (1 + 1)- and two-dimensional topological insulators, we suggest that nontrivial spin-orbital dynamics may accompany anomalous quantum charge Hall states.