ArticleACS nano2026
Vibrational Disorder Effects on Temperature-Resolved X-Ray Absorption Signatures of Metal Catalysts: From Single-Atoms to Clusters and Nanoparticles.
Article in ACS nano, 2026. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Not yet cited in PubMed.
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Abstract
Revealing dynamic local-structure changes of (sub)nanometric metal species under operating conditions is essential. In heterogeneous catalysis, this insight enables the rationalization of operation and optimization of catalyst efficiency and stability. Extended X-ray absorption fine structure (EXAFS) provides element-specific access to metal-metal coordination numbers, interatomic distances, and local disorder, which is pivotal when active motifs lack long-range order. Yet, accurate determination of structural parameters from EXAFS signatures is often complicated by the convolution of static heterogeneity and thermal vibration effects, encoded in the Debye-Waller factor:
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