Biomimetic supported catalyst inspired by stalked crinoid.

Can Liao, Shunjie Liu, Qingxian Kuang, Ruoyu Zhang, Chunwei Zhuo, Zhaoyan Sun, Xuesi Chen, Xianhong Wang

Abstract read

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Article in Nature communications, 2026. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Not yet cited in PubMed.

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1 · What the graph read from it

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4 · The record

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5 · Who and what money

Authors and funding

8 authors.

Can LiaoState Key Laboratory of Polymer Science and Technology, Changchun Institute of Applied Chemistry, Chinese Academy of Sciences, Changchun, Jilin, China.ORCID http://orcid.org/0009-0000-3994-7216

Shunjie LiuState Key Laboratory of Polymer Science and Technology, Changchun Institute of Applied Chemistry, Chinese Academy of Sciences, Changchun, Jilin, China. sjliu@ciac.ac.cn.ORCID http://orcid.org/0000-0001-5514-0738

Qingxian KuangState Key Laboratory of Polymer Science and Technology, Changchun Institute of Applied Chemistry, Chinese Academy of Sciences, Changchun, Jilin, China.

Ruoyu ZhangState Key Laboratory of Polymer Science and Technology, Changchun Institute of Applied Chemistry, Chinese Academy of Sciences, Changchun, Jilin, China.

Chunwei ZhuoState Key Laboratory of Polymer Science and Technology, Changchun Institute of Applied Chemistry, Chinese Academy of Sciences, Changchun, Jilin, China.

Zhaoyan SunState Key Laboratory of Polymer Science and Technology, Changchun Institute of Applied Chemistry, Chinese Academy of Sciences, Changchun, Jilin, China.ORCID http://orcid.org/0000-0002-6357-3039

Xuesi ChenState Key Laboratory of Polymer Science and Technology, Changchun Institute of Applied Chemistry, Chinese Academy of Sciences, Changchun, Jilin, China.ORCID http://orcid.org/0000-0003-3542-9256

Xianhong WangState Key Laboratory of Polymer Science and Technology, Changchun Institute of Applied Chemistry, Chinese Academy of Sciences, Changchun, Jilin, China. xhwang@ciac.ac.cn.ORCID http://orcid.org/0000-0002-4228-705X

Funding

National Natural Science Foundation of China (National Science Foundation of China) 52588201National Natural Science Foundation of China (National Science Foundation of China) U25A20250

6 · The paper itself

Abstract

Supported catalysis is considered as an ideal catalytic mode as it combines the advantages of homogeneous catalysis (activity and selectivity) and heterogeneous catalysis (separation and recyclability). However, its application is greatly limited by the loss of catalytic performance after immobilization of molecular catalyst on supports. Inspired by the upright feeding posture of stalked crinoids-characterized by outstretched arms with ordered pinnules extending away from the substrate-we addressed this issue by immobilizing of a linear polymer catalyst decorated with aluminum porphyrin on silica. Our catalyst demonstrates remarkable productivity (62.4 kg polyols/g Al porphyrin), polymer selectivity (99%) and proton tolerance (320,000 equiv. to [Al]) under highly dilute conditions (0.000125 mol [Al]%, 17.8 ppm) for telomerization of CO

Identifiers

PMID42031820

DOI10.1038/s41467-026-71854-6

PMCPMC13319120

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Read under generation 80e0d062 · epoch 390. Bibliography from PubMed, PubMed Central and OpenAlex; grants from NIH RePORTER; trial links from ClinicalTrials.gov; estimates, votes and beliefs from the OpenQuestion graph.