ArticleACS catalysis2026
Understanding the Propagation Step in a Photoredox Cycloaddition Chain Reaction.
Article in ACS catalysis, 2026. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Not yet cited in PubMed.
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6 authors.
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Abstract
Photoredox catalysis has become increasingly significant in academic and industrial processes, replacing harsh reaction conditions and high temperatures with visible light. Photoredox chain reactions that proceed via dark electron or hole "catalysis" represent an intriguing pathway to achieving high-productivity photoredox reactions. Though photoredox chain reactions are known, our understanding of how to design reactions that exhibit chain behavior remains limited. In particular, a key step in designing a chain reaction is a dark propagation step, where an energetically upconverted electron or hole initiates a subsequent cycle of product generation. This study combines quantum yield (QY) measurements, transient absorption spectroscopy (TAS), electrochemical investigations, kinetic modeling, and computational studies of a ruthenium-catalyzed photoredox chain [4 + 2] cyclization between
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