ArticleMacromolecules2026
Supramolecular Assembly of End-Functionalized Polystyrene and Polydimethylsiloxane with Hybrid Nanostructures.
Article in Macromolecules, 2026. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Not yet cited in PubMed.
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Authors and funding
2 authors.
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Abstract
Blends of oppositely charged polymers are capable of self-assembling into well-ordered nanostructures via supramolecular self-assembly. A series of monosulfonated-terminated polystyrene (PS) and monopiperidine-terminated poly-(dimethylsiloxane) (PDMS) polymers with different molecular weights were synthesized and blended to investigate their phase behavior. A new synthetic route for piperidine-terminated PDMS with low dispersity and high end-group fidelity was developed based on a functionalized initiator accessible from commercially available reagents and compatible with anionic ring-opening polymerization. The resulting nanostructure of the blends was measured via small-angle X-ray scattering (SAXS) performed across a range of temperatures and revealed disordered structures in blends prepared with low molecular weight polymers. A model derived by Tanaka using the random phase approximation (RPA) was applied to extract the heteroassociation fraction (
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Registered trials
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