ArticleACS applied electronic materials2026
Enhanced Piezoelectric Effect in P(VDF-TrFE) through Synergistic Templating by PEDOT:PSS and Paper.
Article in ACS applied electronic materials, 2026. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Not yet cited in PubMed.
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Abstract
To reduce the harm of electronic waste, there is impetus to expand the use of biodegradable substrates, biocompatible materials, and battery-free devices. In this study, a piezoelectric paper composite is produced by integrating polyvinylidene fluoride-trifluoroethylene [P-(VDF-TrFE)] with the conducting polymer poly-(3,4-ethylenedioxythiophene) polystyrenesulfonate (PEDOT:PSS) and wood fiber paper. It is shown that the combined effect of PEDOT:PSS and paper leads to an enhanced out-of-plane piezoelectric coefficient in P-(VDF-TrFE), without the need for electric poling. The enhanced piezoelectric performance arises from a synergistic templating effect of PEDOT:PSS and paper that induces a sharp increase in the population of edge-on β phase P-(VDF-TrFE) crystallites. The templating effect relies on supramolecular interactions between PSS and paper that lead to PEDOT enrichment and a linear PEDOT conformation at the interface with P-(VDF-TrFE). Computational modeling reveals that linear PEDOT promotes β phase PVDF growth over the α phase due to a greater availability of hydrogen bonds. The synergistic templating of P-(VDF-TrFE) on PEDOT:PSS-coated paper opens avenues for tuning the properties of piezoelectric paper.
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