Inert Catalytic Sites Unlocked by Micropollutants for Rapid Water Decontamination with Near-Complete Chemical Utilization.

Yu-Hang Li, Mingyi Liu, Yuanhao Li, Yaran Bai, Fu-Xue Wang, Xiaoyi Hu, Xiaoguang Duan, Haodong Ji

Abstract read

In one paragraph

Article in Advanced materials (Deerfield Beach, Fla.), 2026. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Not yet cited in PubMed.

0numbers the graph read from it

0cells of the map it votes in

0citing papers in PubMed

–field-weighted citation impact

1 · What the graph read from it

What it found

Each row is one number read from the abstract, on the scale the paper reported it, with its interval. Left of the dashed line favours the treatment, right favours the comparator. Under each row is the sentence it came from. New to these charts? A ten-minute tutorial.

The abstract states no effect estimate the extractor could read, or names no intervention and outcome on the map, so this paper lights no cell and moves no belief. It is still indexed, cited and linked below.

2 · The registry

The trial behind it

Trials whose registry record cites this paper, or whose number appears in the abstract. A trial that started after this paper was published is citing it as background, not reporting it.

Neither the registry nor the abstract names a trial number. If this is a trial report, that itself is worth knowing.

3 · Its place in the literature

Who cites it

0 citing papers in PubMed.

No citing paper in PubMed yet.

4 · The record

Corrections and comments

PubMed lists nothing against this paper. Absence here is not a guarantee, only a check that was made.

5 · Who and what money

Authors and funding

8 authors.

Yu-Hang LiEco-environment and Resource Efficiency Research Laboratory, School of Environment and Energy, Peking University Shenzhen Graduate School, Shenzhen, Guangdong, P. R. China.

Mingyi LiuEco-environment and Resource Efficiency Research Laboratory, School of Environment and Energy, Peking University Shenzhen Graduate School, Shenzhen, Guangdong, P. R. China.

Yuanhao LiDepartment of Chemistry, University of Pittsburgh, Pennsylvania, USA.

Yaran BaiEco-environment and Resource Efficiency Research Laboratory, School of Environment and Energy, Peking University Shenzhen Graduate School, Shenzhen, Guangdong, P. R. China.

Fu-Xue WangLaboratory of Agro-Forestry Environmental Processes and Ecological Regulation of Hainan Province, School of Environmental Science and Engineering, Hainan University, Hainan, P. R. China.

Xiaoyi HuEco-environment and Resource Efficiency Research Laboratory, School of Environment and Energy, Peking University Shenzhen Graduate School, Shenzhen, Guangdong, P. R. China.

Xiaoguang DuanSchool of Chemical Engineering, Adelaide University, Adelaide, South Australia, Australia.ORCID https://orcid.org/0000-0001-9635-5807

Haodong JiEco-environment and Resource Efficiency Research Laboratory, School of Environment and Energy, Peking University Shenzhen Graduate School, Shenzhen, Guangdong, P. R. China.

Funding

2023 Shenzhen Sustainable Supporting Funds for Colleges and Universities 20231121170027002National Natural Science Foundation of China 22576005Shenzhen Science and Technology Program JCYJ20241202125900002

6 · The paper itself

Abstract

The utilization efficiencies of peroxide and the evolved reactive species are typically low in advanced oxidation processes due to their self-quenching or scavenging by background factors in water matrices. Here, we design a new Co-based metal-organic framework (PKU-24) with a six-coordinate structure that induces strong electron localization and suppresses the redox activity of Co sites, thereby blocking the electron-transfer pathway. Interestingly, electron-rich pollutants with oriented dipole moments can act as molecular "switches", effectively turning on PKU-24 activity for peroxymonosulfate (PMS) activation. Computations reveal that the dipole moment of pollutants is the decisive descriptor governing the behavior of organic contaminants in activating inert Co centers and reopening the electron-transfer channel to mediate SO

Indexed as

charge‐confined PKU‐24dipole momentperoxymonosulfate activationpollutant degradationsinglet oxygen

Identifiers

PMID42003025

DOI10.1002/adma.73103

PMCPMC13181517

What OpenQuestion holds

Textmetadata

LicenceCC BY

Read underepoch 390

Registered trials

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Read under generation 80e0d062 · epoch 390. Bibliography from PubMed, PubMed Central and OpenAlex; grants from NIH RePORTER; trial links from ClinicalTrials.gov; estimates, votes and beliefs from the OpenQuestion graph.