ArticleBiomacromolecules2026
Light and Enzymatic Cooperative Response in Supramolecular Fibers: A Synergistic Strategy for Potential Drug Delivery Applications.
Article in Biomacromolecules, 2026. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Not yet cited in PubMed.
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6 authors.
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Abstract
Supramolecular Polymers (SPs) can undergo reversible self-assembly in response to internal or external stimuli. Design strategies based on the benzene-1,3,5-tricarboxamide (BTA) core are gaining increasing attention. In this study, we describe a BTA amphiphile that self-assembles into supramolecular fibers in water and is able to respond to both light and enzymatic activity. An azobenzene moiety (AZB) and Gly-Phe-Leu-Gly amino acid sequence (GFLG) were incorporated into the BTA monomer skeleton to build three identical wedges that respond to light and Cathepsin B activity. The synergistic application of two orthogonal stimuli enabled modulation of the assembly of BTA-AZB-GFLG fibers through the cooperative response to stimuli. These findings provide new insights into the use of SPs for future drug delivery applications.
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