ArticleAdvanced science (Weinheim, Baden-Wurttemberg, Germany)2026
Bipolar Covalent Organic Frameworks Crafting Core-Shell Heterostructured Cathode for High-Performance Lithium-Organic Batteries.
Article in Advanced science (Weinheim, Baden-Wurttemberg, Germany), 2026. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Not yet cited in PubMed.
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Abstract
Covalent organic frameworks (COFs) with tunable molecular structures and ordered porous channels have emerged as promising cathode materials for lithium-organic batteries. However, their practical application is still hindered by low operating voltages, limited specific capacities, and sluggish charge transport kinetics. In this work, a new carbon nanotube@bipolar COF (CNT@COF) core-shell heterostructure cathode was rationally crafted through the synergistic integration of molecular and microstructural engineering. The robust 3D hybrid architecture features a conductive CNT core and COF shells enriched with p-/n-type nitrogen electroactive sites, enabling rapid electron/ion transport while maximizing electrochemical utilization. Consequently, the CNT@COF cathode exhibits a high reversible capacity of 226.5 mAh g
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