ArticleJournal of the American Society for Mass Spectrometry2026
Experimental and Computational Investigation of Sulfur Chemistry in the DART-MS Gas Stream: Implications for the Interpretation of the Mass Spectra of Organic Disulfides.
Article in Journal of the American Society for Mass Spectrometry, 2026. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Not yet cited in PubMed.
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Abstract
Direct analysis in real time-high-resolution mass spectrometry (DART-HRMS) has proven useful for the detection and faithful representation of labile organosulfur compounds (OSCs). Nevertheless, it has been found that when exposed to the metastable helium (He*) of the DART gas stream under soft ionization conditions, some classes of OSCs such as disulfides, undergo several reactions to produce new organosulfur species, which complicate interpretation of their spectra. In this work, these new entities were characterized and the mechanisms of their formation explored. DART-HRMS analysis of diphenyl disulfide (PhSSPh) exhibited peaks consistent with [PhSSPh]
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