ArticleACS polymers Au2026
Introduction of Self-Healing and Recyclable Properties into Functionalized Polyisoprene Rubber via Thiol-Ene Reaction.
Article in ACS polymers Au, 2026. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Not yet cited in PubMed.
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Abstract
Covalently cross-linked rubbers face persistent sustainability challenges due to their irreversible networks hindering recycling, while polarity mismatch complicates the incorporation of additional self-healing materials into vulcanization-free cis-1,4-polyisoprene (PI). To advance the sustainable development of functionalized PI with additional new features while promoting the elasticity and mechanical properties, our group proposes a straightforward one-step free radical-mediated thiol-ene reaction using l-cysteine (LC) as a biodegradable compound that bears three main functional groups consisting of thiol, carboxylic acid, and amine. The thiol group is covalently attached to the PI double bonds via free radical thiol-ene chemistry, while the carboxylic acid and amine groups facilitate noncovalent cross-linking through dynamic hydrogen bonds. As the LC content increases, the functionalized PI-LC-X (with
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