ArticleACS sustainable chemistry & engineering2024
Catalytic and Inhibitory Effects Induced by Noncovalent Interactions between Cellulose and Lignin during Fast Pyrolysis.
Article in ACS sustainable chemistry & engineering, 2024. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Not yet cited in PubMed.
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Abstract
Biomass fast pyrolysis has emerged as a highly promising technology for producing renewable fuels and chemicals. However, the inherent multiscale and multiphase nature of the process and the heterogeneous nature of biomass feedstocks typically lead to low selectivity toward each bio-oil molecule, posing significant commercialization challenges. A molecular-level understanding of the biomass pyrolysis reaction kinetics considering the interactions between the main constituents (i.e., cellulose, hemicellulose, and lignin) is essential to advance the macroscopic design, scale-up, and optimization of the process. In this work, microreactor experiments were conducted to determine the effects of lignin structures on the yields of cellulose-derived products during pyrolysis. We show that levoglucosan formation is inhibited by the β-
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