ArticleThe journal of physical chemistry letters2026
Reservoir Dynamics in Vibrational Polaritons Revealed by Detuning-Dependent Ultrafast Spectroscopy.
Article in The journal of physical chemistry letters, 2026. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Not yet cited in PubMed.
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Abstract
There is an emerging consensus that transient spectral features of cavity vibrational polaritons are dominated by molecular population dynamics of the optically dark reservoir rather than by excited-state transitions within the polariton manifold. In this work, we use ultrafast mid-infrared pump-probe spectroscopy to study vibrational polaritons of ammonium thiocyanate (NH
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