ArticleACS applied materials & interfaces2026
From Dead Lithium to Functional Fillers: An in Situ Conversion Strategy for High-Performance All-Solid-State Lithium Metal Batteries.
Article in ACS applied materials & interfaces, 2026. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Not yet cited in PubMed.
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Abstract
Poly(ethylene oxide) (PEO) solid electrolytes offer great promise to realize all-solid-state lithium metal batteries with both high energy density and safety. However, it remains challenging to fabricate ultrathin PEO-based solid electrolytes that can operate at practical current densities with a long lifespan. Here, we develop a 19 μm-thick PEO-based solid electrolyte with a porous polyethylene support, which provides mechanical strength and blocks lithium dendrites. By repeatedly plating and stripping lithium at a high current density and low areal capacity, we ingeniously transform otherwise detrimental "dead lithium" into functional fillers within the PEO solid electrolytes. Results show that LiOH, Li
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