ArticleAdvanced science (Weinheim, Baden-Wurttemberg, Germany)2026
Multifunctional Eutectic Mixtures Enable Integrated Recovery of U, Pu, and Sr From Nuclear Waste.
Article in Advanced science (Weinheim, Baden-Wurttemberg, Germany), 2026. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Not yet cited in PubMed.
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Abstract
Addressing the challenges of nuclear waste management and strategic resource recovery necessitates novel functional materials for the integrated and efficient capture of critical elements. This work reports a class of multifunctional eutectic mixtures (EMs) constructed from crown ether (hydrogen-bond acceptor, HBA) and partially esterified organophosphorus acids (hydrogen-bond donor, HBD). This design integrates the high selectivity of crown ether toward Sr(II) with the strong affinity of organophosphorus ligands for U(VI)/Pu(IV), achieving unprecedented single-step extraction efficiencies exceeding 99.9% for U(VI), 99.8% for Pu(IV), and 99% for Sr(II) under extreme and nearly realistic conditions. This exceptional performance originates from the differentiated metal coordination of crown ether and phosphoric esters, coupled with a synergistic "coordination-encapsulation" effect mediated by the formation of reverse micellar supramolecular structures. Our findings not only provide high-performance materials for the simultaneous recovery of critical radionuclides but also demonstrate the great potential of EMs as a sustainable platform for addressing complex separation scenarios.
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