ArticleInorganic chemistry2026
Multifunctional Photocatalysts Based on Half-Sandwich Cyclometalated Ir(III) Complexes with π-Extended Ligands.
Article in Inorganic chemistry, 2026. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Not yet cited in PubMed.
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Abstract
Photocatalysis has emerged as a powerful strategy in synthetic organic chemistry to avoid harsh conditions and toxic oxidants. Herein, we report the photocatalytic activity of half-sandwich Ir(III) complexes in different transformations. For the first time, Cp*Ir(III) complexes were applied in photooxidative coupling reactions of amines, without any additives, achieving quantitative imine formation, and in thioether photooxidation reactions, reaching high chemoselectivity for sulfoxide formation. Furthermore, exceptional activity was observed in photodehydrogenation of N-heterocyclic substrates. Reactions proceeded under mild conditions, including room temperature and an ambient air or oxygen atmosphere, with considerably low catalyst loadings (0.005-0.25 mol %). Complex
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