Triggering dynamically disordered lithium sublattice in superionic conductors.

Chaohong Guan, Jiawei Zong, Jiacong Li, Runxin Ouyang, Yifeng Zhao, Fuqiang Huang, Hong Zhu

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Article in Nature communications, 2026. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Not yet cited in PubMed.

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7 authors.

Chaohong Guan *University of Michigan-Shanghai Jiao Tong University Joint Institute, Shanghai Jiao Tong University, Shanghai, China.

Jiawei Zong *Key Lab of Intelligent Creation for Extreme Energy Materials of Ministry of Education, Shanghai Jiao Tong University, Shanghai, China.

Jiacong LiShanghai Institute of Ceramics, Chinese Academy of Sciences, Shanghai, China.

Runxin OuyangUniversity of Michigan-Shanghai Jiao Tong University Joint Institute, Shanghai Jiao Tong University, Shanghai, China.

Yifeng ZhaoShanghai Institute of Ceramics, Chinese Academy of Sciences, Shanghai, China.

Fuqiang HuangKey Lab of Intelligent Creation for Extreme Energy Materials of Ministry of Education, Shanghai Jiao Tong University, Shanghai, China. huangfq@sjtu.edu.cn.

Hong ZhuUniversity of Michigan-Shanghai Jiao Tong University Joint Institute, Shanghai Jiao Tong University, Shanghai, China. hong.zhu@sjtu.edu.cn.ORCID http://orcid.org/0000-0001-7919-5661

Funding

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6 · The paper itself

Abstract

The design of superionic conductors has been largely focused on static structural features, with the dynamic ion transport mechanism less explored. Here, we explore a paradigm that harnesses the polyanion rotations to trigger the dynamically disordered Li sublattice as well as the liquid-like cation diffusion for superior ionic conductivity in crystals. A descriptor called rotation tolerance factor was proposed as a predictive metric for identifying the potential fast-rotating anion clusters with the low mass and reduced valence charge for given structural frameworks. Guided by this factor, halides with rotational polyanions, namely Li

Identifiers

PMID41917061

DOI10.1038/s41467-026-71304-3

PMCPMC13201799

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