ArticleChemical science2026
Solvation-driven interphase engineering and mechanical failure pathways in large-scale anode-free lithium metal batteries.
Article in Chemical science, 2026. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Not yet cited in PubMed.
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Authors and funding
5 authors.
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Abstract
Anode-free lithium-metal batteries promise ultrahigh energy density but remain limited by unstable interfaces and safety concerns. Here, we demonstrate that fluorinated-ether solvation chemistry directly dictates interphase formation, thermal behavior, and performance in large-format Cu‖NMC90 cells. We reveal that introducing 1,1,2,2-tetrafluoroethyl 2,2,3,3-tetrafluoropropyl ether (TTE) into a localized high-concentration electrolyte restructures the Li
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