ArticleNature communications2026
Decoupling charge‒discharge electrolysis for hydrogen evolution and organic oxidation reactions.
Article in Nature communications, 2026. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Not yet cited in PubMed.
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Abstract
Replacing the oxygen evolution reaction with more thermodynamically favourable organic oxidation reactions (OORs) can enable energy-efficient hydrogen evolution and hydrogenation. However, cathodic reduction rates are limited by sluggish OORs. Herein, we report a decoupled electrolysis strategy using a solid redox reservoir (RR) to realize an optimized hydrogen evolution reaction (HER) paired with valuable chemical synthesis. The decoupled system with a rechargeable capability features a HER coupled with RR oxidation for electricity storage, which is followed by the conversion of OORs (e.g., ethylene glycol, glycerol) into value-added chemicals coupled with the reduction of the oxidized RR to generate electricity. The fast kinetics of RR oxidation and membrane-free cell operation optimize the HER rate. The value-added chemicals and electricity are cocreated during the discharge process, offering more economic benefits. This decoupling design is universally applicable to other OORs-paired reduction systems (e.g., acetylene-to-ethylene semihydrogenation) to synthesize various chemicals for electricity storage and generation, paving a sustainable avenue for H
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