ArticleACS applied materials & interfaces2026
Free-Standing Boron-Doped Graphene Hydrogel Buckypaper Fabricated via Zinc-Plate Reduction for High-Performance Supercapacitors.
Article in ACS applied materials & interfaces, 2026. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Not yet cited in PubMed.
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Abstract
Graphene offers exceptional mechanical flexibility and superior electrical conductivity that are highly desirable for next-generation supercapacitors; however, its intrinsic strong π-π stacking interactions severely hinder energy-storage performance by blocking active redox sites and restricting ion-accessible pathways. To address these limitations, we developed a binder-free, free-standing, boron-doped graphene hydrogel buckypaper with a hierarchical architecture. In this study, a mixed suspension of thermally activated boron-doped expanded graphene (BT-rGO) and graphene oxide (GO) was integrated via a redox reaction using a Zn plate as a substrate, enabling the instantaneous fabrication of a free-standing BT-rGO/Zn-rGO hydrogel buckypaper. The boron-doped graphene framework exhibits enhanced wettability, facilitating efficient electrolyte ion transportation, while the heteroatom-induced uneven charge distribution modulates the local electronegativity and improves electroconductivity throughout the free-standing hydrogel buckypaper network. The electrochemically enhanced E-BT-rGO
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