ArticleAngewandte Chemie (International ed. in English)2026
MOFs as New Catalytic Platform for Covalent Adaptable Networks: Catalysis Meets Reinforcement.
Article in Angewandte Chemie (International ed. in English), 2026. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Not yet cited in PubMed.
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Abstract
Catalysis of bond exchange reactions is a versatile route to adjust kinetics and onset temperature of bond exchange reactions in covalent adaptable networks (CANs). In this work, we introduce a novel heterogeneous catalytic platform for CANs by immobilizing bases of low molecular weight on metal organic frameworks (MOFs). Specifically, the base 1,5,7-triazabicyclo(4.4.0)dec-5-ene (TBD) was coordinated on the MOF UiO-66. The obtained catalyst UiO-TBD benefits from the high loading capacity of the MOF and exhibits similar catalytic activity in accelerating thiol-thioester exchange reactions in dynamic photopolymers compared to free TBD while outperforming non-porous heterogeneous systems using ZrO
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