ArticleChemical science2026
Temperature orthogonal dynamic polymer networks.
Article in Chemical science, 2026. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Not yet cited in PubMed.
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9 authors.
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Abstract
Latent catalysts have gained increased attention for balancing high creep resistance with rapid (re)processability in covalent adaptable polymer networks (CANs). Among the reported systems, thermolatent catalysts offer particular advantages, as their activation is independent of part geometry, optical transparency, or irradiation depth, making them highly attractive for bulk materials and additively manufactured components. Here, a systematic study of thermobase generators (TBGs) with distinct activation and deactivation temperatures is presented, and their impact on bond-exchange-controlled stress relaxation in dynamic thiol-ene photopolymers undergoing transesterification is quantitatively assessed. Cyanoacetate- and oxalate-based TBGs, releasing amine bases at well-separated temperature windows, are investigated to directly correlate catalyst (de)activation with macroscopic flow behavior. Based on their non-overlapping thermal profiles, a cyanoacetate-based TBG releasing
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