ArticleAngewandte Chemie (International ed. in English)2026
Ammonia-Induced Metal-Organic Framework Membrane Pore Tuning for Hydrogen Separation.
Article in Angewandte Chemie (International ed. in English), 2026. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Not yet cited in PubMed.
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10 authors.
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Abstract
Ammonia has attracted great attention as a key material for clean hydrogen production, such as the ammonia cracking process. Remaining trace ammonia in the purification step is considered a critical impurity due to its toxic and corrosive nature. Herein, we introduce ammonia as a tuning agent for MOF membranes to control their gas transport behavior. When exposed to ammonia, the ZIF-8 membrane undergoes partial surface amorphization due to strong interactions between ammonia and the framework, while the adjacent ZIF-8 region becomes rigid. As a result, the ammonia-treated ZIF-8 membrane exhibits the intrinsic gas-selective property rather than the flexible one, yielding excellent H
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