ArticleLight, science & applications2026
In-situ formation of oriented perovskite nanosheets with tailored optical dipoles enabling >30% EQE in pure-red LEDs.
Article in Light, science & applications, 2026. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 2 papers.
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Who cites it
2 citing papers in PubMed.
- Perovskite Light-Emitting Diodes: Engineering, Stability, and Applications.Micromachines · 2026Review
- Compositional Homogenization and Dielectric Modulation of Pb/Sr Mixed Perovskites for Efficient and Bright Deep-Blue Light-Emitting Diodes.Advanced materials (Deerfield Beach, Fla.) · 2026Article
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Authors and funding
18 authors.
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Abstract
The integration of crystallographic control into solution-processed perovskite films remains a challenge for efficient light emission, as disordered optical dipoles fundamentally limit photon extraction, a bottleneck constraining both classical and quantum planar optoelectronic devices. Here, we address this by developing an in situ formation strategy for oriented quasi-2D perovskite nanosheets within films via ligand-engineered crystallization. By designing and orchestrating steric hindrance and π-π interactions of ligands, we direct the crystallization kinetics to yield regular face-on nanosheets exhibiting enhanced horizontal transition dipole moment orientation compared to conventional isotropic films. The in situ architectural control also elevates both the photoluminescence quantum yield beyond 90% and carrier mobility comparable to 3D perovskite levels. These synergies enable perovskite light-emitting diodes (PeLEDs) with an external quantum efficiency (EQE) of 31.2% for pure-red emission at 635 nm, comparing favorably to other pure-red PeLEDs. Concurrently, the peak luminance and operational stability of the in situ nanosheet PeLEDs exhibit significant improvements.
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Registered trials
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