ArticleRSC advances2026
Length-dependent quantum interference and high thermoelectric response ferrocene-modified OPE wires.
Article in RSC advances, 2026. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Not yet cited in PubMed.
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Abstract
We present a study of the length-dependent charge transport properties of a homologous series of oligo(phenylene-ethynylene) (OPE) molecular wires integrated with ferrocene units (Fe 1-Fe 5). Theoretical analysis reveals a coherent, length-dependent transport mechanism governed by quantum interference, with a distinct odd-even parity effect. Molecules with an odd number of ferrocene units exhibit a characteristic transmission dip within the HOMO-LUMO gap, a signature of destructive quantum interference (DQI), while even-numbered molecules show constructive quantum interference (CQI). This demonstrates that the interference behaviour is a holistic property of the full molecular length, not merely of the ferrocene core. The series exhibits efficient long-range tunneling, with a decay constant of
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