ArticleNature communications2026
Multicomponent solid-solution alloy negative electrode for Li-metal batteries.
Article in Nature communications, 2026. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Not yet cited in PubMed.
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19 authors.
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Abstract
Lithium metal batteries possess the high theoretical specific energy owing to the high theoretical specific capacity of lithium metal. However, practical implementations necessitate a reduction in both lithium mass fraction and lithium utilization within the negative electrode to enhance cycling life and suppress dendrite formation, resulting in a practical reversible capacity of only 30 - 50% of the theoretical value. Herein, we present a lithium metal-based multicomponent solid-solution alloy comprising approximately 90 wt.% lithium, with equal atomic ratios of cadmium, silver, magnesium, and aluminium constituting the remaining 10 wt.%. The increased mixing entropy enables high lithium-atom diffusivity, facilitating inward lithium transport into the metal foil rather than the surface deposition typically observed in conventional lithium metal negative electrodes, while simultaneously promoting a thermodynamically stable (110) crystal facet. These factors collectively yield a dendrite-free negative electrode with a reversible specific capacity of 3100 mAh g
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